Código fuente para qiskit_nature.second_q.problems.electronic_structure_result

# This code is part of a Qiskit project.
#
# (C) Copyright IBM 2020, 2023.
#
# This code is licensed under the Apache License, Version 2.0. You may
# obtain a copy of this license in the LICENSE.txt file in the root directory
# of this source tree or at http://www.apache.org/licenses/LICENSE-2.0.
#
# Any modifications or derivative works of this code must retain this
# copyright notice, and modified files need to carry a notice indicating
# that they have been altered from the originals.

"""The electronic structure result."""

from __future__ import annotations

from functools import reduce
from typing import TYPE_CHECKING, Dict, List, Optional, Tuple, cast

import numpy as np

from qiskit_nature.constants import DEBYE

from .eigenstate_result import EigenstateResult

if TYPE_CHECKING:
    from qiskit_nature.second_q.properties import ElectronicDensity

# A dipole moment, when present as X, Y and Z components will normally have float values for all
# the components. However when using Z2Symmetries, if the dipole component operator does not
# commute with the symmetry then no evaluation is done and None will be used as the 'value'
# indicating no measurement of the observable took place
DipoleTuple = Tuple[Optional[float], Optional[float], Optional[float]]


[documentos]class ElectronicStructureResult(EigenstateResult): """The electronic structure result.""" def __init__(self) -> None: super().__init__() self._hartree_fock_energy: float = 0.0 self._nuclear_repulsion_energy: Optional[float] = None self._nuclear_dipole_moment: Optional[DipoleTuple] = None self._computed_energies: Optional[np.ndarray] = None self._computed_dipole_moment: Optional[List[DipoleTuple]] = None self._extracted_transformer_energies: Dict[str, float] = {} self._extracted_transformer_dipoles: Optional[List[Dict[str, DipoleTuple]]] = None self._reverse_dipole_sign: bool = False self._num_particles: Optional[List[float]] = None self._magnetization: Optional[List[float]] = None self._total_angular_momentum: Optional[List[float]] = None self._electronic_density: "ElectronicDensity" | None = None @property def hartree_fock_energy(self) -> float: """Returns Hartree-Fock energy""" return self._hartree_fock_energy @hartree_fock_energy.setter def hartree_fock_energy(self, value: float) -> None: """Sets Hartree-Fock energy""" self._hartree_fock_energy = value @property def nuclear_repulsion_energy(self) -> Optional[float]: """Returns nuclear repulsion energy when available from driver""" return self._nuclear_repulsion_energy @nuclear_repulsion_energy.setter def nuclear_repulsion_energy(self, value: float) -> None: """Sets nuclear repulsion energy""" self._nuclear_repulsion_energy = value @property def nuclear_dipole_moment(self) -> Optional[DipoleTuple]: """Returns nuclear dipole moment X,Y,Z components in A.U when available from driver""" return self._nuclear_dipole_moment @nuclear_dipole_moment.setter def nuclear_dipole_moment(self, value: DipoleTuple) -> None: """Sets nuclear dipole moment in A.U""" self._nuclear_dipole_moment = value # TODO we need to be able to extract the statevector or the optimal parameters that can # construct the circuit of the GS from here (if the algorithm supports this) @property def total_energies(self) -> Optional[np.ndarray]: """Returns ground state energy if nuclear_repulsion_energy is available from driver""" if self.electronic_energies is None: return None nre = self.nuclear_repulsion_energy if self.nuclear_repulsion_energy is not None else 0 # Adding float to np.ndarray adds it to each entry return self.electronic_energies + nre @property def electronic_energies(self) -> Optional[np.ndarray]: """Returns electronic part of ground state energy""" # TODO the fact that this property is computed on the fly breaks the `.combine()` # functionality # Adding float to np.ndarray adds it to each entry if self.computed_energies is None: return None return self.computed_energies + self.extracted_transformer_energy @property def computed_energies(self) -> Optional[np.ndarray]: """Returns computed electronic part of ground state energy""" return self._computed_energies @computed_energies.setter def computed_energies(self, value: np.ndarray) -> None: """Sets computed electronic part of ground state energy""" self._computed_energies = value @property def extracted_transformer_energies(self) -> Dict[str, float]: """Returns the energies extracted by any applied transformers.""" return self._extracted_transformer_energies @extracted_transformer_energies.setter def extracted_transformer_energies(self, value: Dict[str, float]) -> None: """Sets the energies extracted by any applied transformers.""" self._extracted_transformer_energies = value @property def extracted_transformer_energy(self) -> float: """Returns the sum of all extracted energies.""" return sum(self.extracted_transformer_energies.values()) # Dipole moment results. Note dipole moments of tuples of X, Y and Z components. Chemistry # drivers either support dipole integrals or not. Note that when using Z2 symmetries of
[documentos] def has_dipole(self) -> bool: """Returns whether dipole moment is present in result or not""" return self.nuclear_dipole_moment is not None and self.electronic_dipole_moment is not None
@property def reverse_dipole_sign(self) -> bool: """Returns if electronic dipole moment sign should be reversed when adding to nuclear""" return self._reverse_dipole_sign @reverse_dipole_sign.setter def reverse_dipole_sign(self, value: bool) -> None: """Sets if electronic dipole moment sign should be reversed when adding to nuclear""" self._reverse_dipole_sign = value @property def total_dipole_moment(self) -> Optional[List[float]]: """Returns total dipole of moment""" if self.dipole_moment is None: return None # No dipole at all tdm: List[float] = [] for dip in self.dipole_moment: if np.any(np.equal(list(dip), None)): tdm.append(None) # One or more components in the dipole is None else: tdm.append(np.sqrt(np.sum(np.power(list(dip), 2)))) return tdm @property def total_dipole_moment_in_debye(self) -> Optional[List[float]]: """Returns total dipole of moment in Debye""" tdm = self.total_dipole_moment if tdm is None: return None return [dip / DEBYE if dip is not None else None for dip in tdm] @property def dipole_moment(self) -> Optional[List[DipoleTuple]]: """Returns dipole moment""" edm = self.electronic_dipole_moment if edm is None: return None nrd = self.nuclear_dipole_moment if self.nuclear_dipole_moment is not None else (0, 0, 0) if self.reverse_dipole_sign: edm = [ cast(DipoleTuple, tuple(-1 * x if x is not None else None for x in dip)) for dip in edm ] return [_dipole_tuple_add(dip, nrd) for dip in edm] @property def dipole_moment_in_debye(self) -> Optional[List[DipoleTuple]]: """Returns dipole moment in Debye""" dipm = self.dipole_moment if dipm is None: return None dipmd = [] for dip in dipm: dipmd0 = dip[0] / DEBYE if dip[0] is not None else None dipmd1 = dip[1] / DEBYE if dip[1] is not None else None dipmd2 = dip[2] / DEBYE if dip[2] is not None else None dipmd += [(dipmd0, dipmd1, dipmd2)] return dipmd @property def electronic_dipole_moment(self) -> Optional[List[DipoleTuple]]: """Returns electronic dipole moment""" if self.computed_dipole_moment is None or self.extracted_transformer_dipoles is None: return None return [ _dipole_tuple_add(comp_dip, extr_dip) for comp_dip, extr_dip in zip( self.computed_dipole_moment, self.extracted_transformer_dipole ) ] @property def computed_dipole_moment(self) -> Optional[List[DipoleTuple]]: """Returns computed electronic part of dipole moment""" return self._computed_dipole_moment @computed_dipole_moment.setter def computed_dipole_moment(self, value: List[DipoleTuple]) -> None: """Sets computed electronic part of dipole moment""" self._computed_dipole_moment = value @property def extracted_transformer_dipoles(self) -> Optional[List[Dict[str, DipoleTuple]]]: """Returns the dipole moments extracted by any applied transformers.""" return self._extracted_transformer_dipoles @extracted_transformer_dipoles.setter def extracted_transformer_dipoles(self, value: List[Dict[str, DipoleTuple]]) -> None: """Sets the dipole moments extracted by any applied transformers.""" self._extracted_transformer_dipoles = value @property def extracted_transformer_dipole(self) -> List[DipoleTuple]: """Returns the sum of all extracted dipole moments.""" extracted_dips = self.extracted_transformer_dipoles if extracted_dips is None: return [] extracted_dipms = [] for dipm in self.extracted_transformer_dipoles: if not dipm: extracted_dipms.append(cast(DipoleTuple, (0, 0, 0))) else: extracted_dipms.append(reduce(_dipole_tuple_add, dipm.values())) return extracted_dipms # Other measured operators. If these are not evaluated then None will be returned # instead of any measured value.
[documentos] def has_observables(self): """Returns whether result has aux op observables such as spin, num particles""" return ( self.total_angular_momentum is not None or self.num_particles is not None or self.magnetization is not None )
@property def total_angular_momentum(self) -> Optional[List[float]]: """Returns total angular momentum (S^2)""" return self._total_angular_momentum @total_angular_momentum.setter def total_angular_momentum(self, value: List[float]) -> None: """Sets total angular momentum""" self._total_angular_momentum = value @property def spin(self) -> Optional[List[float]]: """Returns computed spin""" if self.total_angular_momentum is None: return None spin = [] for total_angular_momentum in self.total_angular_momentum: spin.append((-1.0 + np.sqrt(1 + 4 * total_angular_momentum)) / 2) return spin @property def num_particles(self) -> Optional[List[float]]: """Returns measured number of particles""" return self._num_particles @num_particles.setter def num_particles(self, value: List[float]) -> None: """Sets measured number of particles""" self._num_particles = value @property def magnetization(self) -> Optional[List[float]]: """Returns measured magnetization""" return self._magnetization @magnetization.setter def magnetization(self, value: List[float]) -> None: """Sets measured magnetization""" self._magnetization = value @property def electronic_density(self) -> "ElectronicDensity" | None: """Returns the measured electronic density.""" return self._electronic_density @electronic_density.setter def electronic_density(self, electronic_density: "ElectronicDensity" | None) -> None: """Sets the measured electronic density.""" self._electronic_density = electronic_density def __str__(self) -> str: """Printable formatted result""" return "\n".join(self.formatted())
[documentos] def formatted(self) -> List[str]: """Formatted result as a list of strings""" lines = [] lines.append("=== GROUND STATE ENERGY ===") lines.append(" ") if self.electronic_energies is not None: lines.append( "* Electronic ground state energy (Hartree): " f"{_complex_to_string(self.electronic_energies[0], self.formatting_precision)}" ) lines.append( " - computed part: " f"{_complex_to_string(self.computed_energies[0], self.formatting_precision)}" ) for name, value in self.extracted_transformer_energies.items(): lines.append( f" - {name} extracted energy part: " f"{_complex_to_string(value, self.formatting_precision)}" ) if self.nuclear_repulsion_energy is not None: lines.append( "~ Nuclear repulsion energy (Hartree): " f"{_complex_to_string(self.nuclear_repulsion_energy, self.formatting_precision)}" ) lines.append( "> Total ground state energy (Hartree): " f"{_complex_to_string(self.total_energies[0], self.formatting_precision)}" ) if self.computed_energies is not None and len(self.computed_energies) > 1: lines.append(" ") lines.append("=== EXCITED STATE ENERGIES ===") lines.append(" ") for idx, (elec_energy, total_energy) in enumerate( zip(self.electronic_energies[1:], self.total_energies[1:]) ): lines.append(f"{(idx + 1): 3d}: ") lines.append( "* Electronic excited state energy (Hartree): " f"{_complex_to_string(elec_energy, self.formatting_precision)}" ) lines.append( "> Total excited state energy (Hartree): " f"{_complex_to_string(total_energy, self.formatting_precision)}" ) if self.has_observables(): lines.append(" ") lines.append("=== MEASURED OBSERVABLES ===") lines.append(" ") for idx, (num_particles, spin, total_angular_momentum, magnetization,) in enumerate( zip( self.num_particles, self.spin, self.total_angular_momentum, self.magnetization, ) ): line = f"{idx: 3d}: " if num_particles is not None: line += f" # Particles: {num_particles:.3f}" if spin is not None: line += f" S: {spin:.3f}" if total_angular_momentum is not None: line += f" S^2: {total_angular_momentum:.3f}" if magnetization is not None: line += f" M: {magnetization:.3f}" lines.append(line) if self.has_dipole(): lines.append(" ") lines.append("=== DIPOLE MOMENTS ===") lines.append(" ") if self.nuclear_dipole_moment is not None: lines.append( "~ Nuclear dipole moment (a.u.): " f"{_dipole_to_string(self.nuclear_dipole_moment, self.formatting_precision)}" ) lines.append(" ") for idx, (elec_dip, comp_dip, extr_dip, dip, tot_dip, dip_db, tot_dip_db,) in enumerate( zip( self.electronic_dipole_moment, self.computed_dipole_moment, self.extracted_transformer_dipoles, self.dipole_moment, self.total_dipole_moment, self.dipole_moment_in_debye, self.total_dipole_moment_in_debye, ) ): lines.append(f"{idx: 3d}: ") lines.append( " * Electronic dipole moment (a.u.): " f"{_dipole_to_string(elec_dip, self.formatting_precision)}" ) lines.append( " - computed part: " f"{_dipole_to_string(comp_dip, self.formatting_precision)}" ) for name, ex_dip in extr_dip.items(): lines.append( f" - {name} extracted energy part: " f"{_dipole_to_string(ex_dip, self.formatting_precision)}" ) if self.nuclear_dipole_moment is not None: lines.append( " > Dipole moment (a.u.): " f"{ _dipole_to_string(dip, self.formatting_precision)} " f"Total: {_complex_to_string(tot_dip, self.formatting_precision)}" ) lines.append( " (debye): " f"{_dipole_to_string(dip_db, self.formatting_precision)} " f"Total: {_complex_to_string(tot_dip_db, self.formatting_precision)}" ) lines.append(" ") return lines
def _dipole_tuple_add(x: Optional[DipoleTuple], y: Optional[DipoleTuple]) -> Optional[DipoleTuple]: """Utility to add two dipole tuples element-wise for dipole additions""" if x is None or y is None: return None return _element_add(x[0], y[0]), _element_add(x[1], y[1]), _element_add(x[2], y[2]) def _element_add(x: Optional[float], y: Optional[float]): """Add dipole elements where a value may be None then None is returned""" return x + y if x is not None and y is not None else None def _dipole_to_string(dipole: DipoleTuple, precision: int = 8): value = "[" for i, dip in enumerate(dipole): value += _complex_to_string(dip, precision) if dip is not None else "None" value += " " if i < len(dipole) - 1 else "]" return value def _complex_to_string(value: Optional[complex], precision: int = 8) -> str: if value is None: return "None" else: real = ( "0.0" if round(value.real, precision) == 0 else ("{:." + str(precision) + "f}").format(value.real).rstrip("0") ) imag = ( "" if round(value.imag, precision) == 0 else ("{:." + str(precision) + "f}").format(value.imag).rstrip("0") + "j" ) string = real if imag != "" and value.imag > 0: string += "+" + imag elif imag != "" and value.imag < 0: string += imag return string